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The Resource Operando research in heterogeneous catalysis, Joost Frenken, Irene Groot, editors

Operando research in heterogeneous catalysis, Joost Frenken, Irene Groot, editors

Editor
Contributor
Summary
This book is devoted to the emerging field of techniques for visualizing atomic-scale properties of active catalysts under actual working conditions, i.e. high gas pressures and high temperatures. It explains how to understand these observations in terms of the surface structures and dynamics and their detailed interplay with the gas phase. This provides an important new link between fundamental surface physics and chemistry, and applied catalysis. The book explains the motivation and the necessity of operando studies, and positions these with respect to the more traditional low-pressure investigations on the one hand and the reality of industrial catalysis on the other. The last decade has witnessed a rapid development of new experimental and theoretical tools for operando studies of heterogeneous catalysis. The book has a strong emphasis on the new techniques and illustrates how the challenges introduced by the harsh, operando conditions are faced for each of these new tools. Therefore, one can also read this book as a collection of recipes for the development of operando instruments. At present, the number of scientific results obtained under operando conditions is still limited and mostly focused on a simple test reaction, the catalytic oxidation of CO. This reaction thus forms a natural binding element between the chapters, linking the demonstrations of new techniques, and also connecting the theoretical and experimental studies. Some first results on other reactions are also presented. If there is one thing that can be concluded already in this early stage, it is that the catalytic conditions themselves can have dramatic effects on the structure and composition of the surfaces of catalysts, which, in turn can greatly affect the mechanisms, the activity, and the selectivity of the chemical reactions that they catalyze.
Language
eng
Work
Publication
Extent
1 online resource.
Contents
  • From the Contents: Scanning probe microscopy under high-pressure conditions
  • Surface X-ray diffraction under high-pressure conditions
  • Ambient pressure X-ray photoelectron spectroscopy
  • Planar laser-induced fluorescence
Isbn
9783319444390
Instance
Label
Operando research in heterogeneous catalysis
Title
Operando research in heterogeneous catalysis
Statement of responsibility
Joost Frenken, Irene Groot, editors
Contributor
Editor
Subject
Language
eng
Summary
This book is devoted to the emerging field of techniques for visualizing atomic-scale properties of active catalysts under actual working conditions, i.e. high gas pressures and high temperatures. It explains how to understand these observations in terms of the surface structures and dynamics and their detailed interplay with the gas phase. This provides an important new link between fundamental surface physics and chemistry, and applied catalysis. The book explains the motivation and the necessity of operando studies, and positions these with respect to the more traditional low-pressure investigations on the one hand and the reality of industrial catalysis on the other. The last decade has witnessed a rapid development of new experimental and theoretical tools for operando studies of heterogeneous catalysis. The book has a strong emphasis on the new techniques and illustrates how the challenges introduced by the harsh, operando conditions are faced for each of these new tools. Therefore, one can also read this book as a collection of recipes for the development of operando instruments. At present, the number of scientific results obtained under operando conditions is still limited and mostly focused on a simple test reaction, the catalytic oxidation of CO. This reaction thus forms a natural binding element between the chapters, linking the demonstrations of new techniques, and also connecting the theoretical and experimental studies. Some first results on other reactions are also presented. If there is one thing that can be concluded already in this early stage, it is that the catalytic conditions themselves can have dramatic effects on the structure and composition of the surfaces of catalysts, which, in turn can greatly affect the mechanisms, the activity, and the selectivity of the chemical reactions that they catalyze.
Member of
Cataloging source
N$T
Dewey number
541/.395
Index
index present
LC call number
QD505
Literary form
non fiction
Nature of contents
  • dictionaries
  • bibliography
http://library.link/vocab/relatedWorkOrContributorName
  • Frenken, Joost W. M.
  • Groot, Irene
Series statement
Springer series in chemical physics
Series volume
volume 114
http://library.link/vocab/subjectName
  • Heterogeneous catalysis
  • Physics
  • Spectroscopy and Microscopy
  • Catalysis
  • Surfaces and Interfaces, Thin Films
  • Physical Chemistry
  • Surface and Interface Science, Thin Films
Label
Operando research in heterogeneous catalysis, Joost Frenken, Irene Groot, editors
Instantiates
Publication
Antecedent source
unknown
Bibliography note
Includes bibliographical references and index
Carrier category
online resource
Carrier category code
  • cr
Carrier MARC source
rdacarrier
Color
multicolored
Content category
text
Content type code
  • txt
Content type MARC source
rdacontent
Contents
From the Contents: Scanning probe microscopy under high-pressure conditions -- Surface X-ray diffraction under high-pressure conditions -- Ambient pressure X-ray photoelectron spectroscopy -- Planar laser-induced fluorescence
Dimensions
unknown
Extent
1 online resource.
File format
unknown
Form of item
online
Isbn
9783319444390
Level of compression
unknown
Media category
computer
Media MARC source
rdamedia
Media type code
  • c
Other control number
10.1007/978-3-319-44439-0
Quality assurance targets
not applicable
Reformatting quality
unknown
Sound
unknown sound
Specific material designation
remote
System control number
ocn967282936
Label
Operando research in heterogeneous catalysis, Joost Frenken, Irene Groot, editors
Publication
Antecedent source
unknown
Bibliography note
Includes bibliographical references and index
Carrier category
online resource
Carrier category code
  • cr
Carrier MARC source
rdacarrier
Color
multicolored
Content category
text
Content type code
  • txt
Content type MARC source
rdacontent
Contents
From the Contents: Scanning probe microscopy under high-pressure conditions -- Surface X-ray diffraction under high-pressure conditions -- Ambient pressure X-ray photoelectron spectroscopy -- Planar laser-induced fluorescence
Dimensions
unknown
Extent
1 online resource.
File format
unknown
Form of item
online
Isbn
9783319444390
Level of compression
unknown
Media category
computer
Media MARC source
rdamedia
Media type code
  • c
Other control number
10.1007/978-3-319-44439-0
Quality assurance targets
not applicable
Reformatting quality
unknown
Sound
unknown sound
Specific material designation
remote
System control number
ocn967282936

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